文献类型：期刊文献

英文题名：From mineralization to low-carbon conversion: emerging paradigms in water decontamination

作者：Cao, Jiazhen[1,2];Qin, Jiewen[1];Fan, Yafei[1];Jiang, Yue[1];Xing, Mingyang[1,2]

机构：[1]East China Univ Sci & Technol, Sch Chem & Mol Engn, Key Lab Green Chem Engn & Ind Catalysis, Shanghai 200237, Peoples R China;[2]East China Univ Sci & Technol, Natl Engn Res Ctr Ind Wastewater Detoxicat & Resou, Shanghai 200237, Peoples R China

年份：2026

卷号：69

期号：4

起止页码：1663

外文期刊名：SCIENCE CHINA-CHEMISTRY

收录：;EI(收录号：20260720059843);WOS:【SCI-EXPANDED(收录号:WOS:001681877000001)】；

基金：This work was supported by the National Key R&D Program of China (SQ2024YFA1211001), the National Natural Science Foundation of China (22325602, 22521201, 22176060, 22406142), the Program of Shanghai Academic/Technology Research Leader (23XD1421000), the Shanghai Municipal Science and Technology Major Project (2018SHZDZX03), the Program of Introducing Talents of Discipline to Universities (B16017) and the Science and Technology Commission of Shanghai Municipality (20DZ2250400).

语种：英文

外文关键词：low-carbon wastewater treatment; selective oxidation; high-value products; controlled polymerization; sustainable-by-design

摘要：The low-carbon conversion of pollutants has emerged as a transformative strategy that bridges environmental remediation with green development, carrying profound implications for achieving carbon neutrality, advancing resource utilization, and promoting a sustainable future. Here, we introduce a conceptual paradigm centered on "carbon transfer", which redefines conventional thinking by moving beyond the complete oxidation of organics into carbon dioxide (CO2). Within this paradigm, the traditional mineralization route is deconstructed into multiple value-driven pathways, including selective oxidation for high-value products, the targeted production of low-carbon small-molecule fuels, and pathways based on the direct oxidative transfer process (DOTP) and organic carbon transfer process (OCTP). This study systematically reviews the key reaction mechanisms and catalyst design strategies involved in each route, with a particular focus on selectivity control methods and scale-up potential, and further proposes forward-looking directions to provide a systematic theoretical foundation and practical technological roadmap for low-carbon wastewater treatment.