文献类型：期刊文献

英文题名：A review of catalytic hydrogenation of carbon dioxide: From waste to hydrocarbons

作者：Cui, Lingrui[1];Liu, Cao[1];Yao, Benzhen[2];Edwards, Peter P.[2];Xiao, Tiancun[2,3];Cao, Fahai[1]

机构：[1]East China Univ Sci & Technol, Engn Res Ctr Large Scale Reactor, Shanghai, Peoples R China;[2]OXCCU Tech Ltd, Ctr Innovat & Enterprise, Begbroke Sci Pk, Oxford, England;[3]Univ Oxford, Dept Chem, Inorgan Chem Lab, Oxford, England

年份：2022

卷号：10

外文期刊名：FRONTIERS IN CHEMISTRY

收录：;WOS:【SCI-EXPANDED(收录号:WOS:000876489600001)】；

语种：英文

外文关键词：catalyst; CO2 hydrogenation; light olefin; hydrocarbon fuels; aromatics; Fischer-Tropsch synthesis

摘要：With the rapid development of industrial society and humankind's prosperity, the growing demands of global energy, mainly based on the combustion of hydrocarbon fossil fuels, has become one of the most severe challenges all over the world. It is estimated that fossil fuel consumption continues to grow with an annual increase rate of 1.3%, which has seriously affected the natural environment through the emission of greenhouse gases, most notably carbon dioxide (CO2). Given these recognized environmental concerns, it is imperative to develop clean technologies for converting captured CO2 to high-valued chemicals, one of which is value-added hydrocarbons. In this article, environmental effects due to CO2 emission are discussed and various routes for CO2 hydrogenation to hydrocarbons including light olefins, fuel oils (gasoline and jet fuel), and aromatics are comprehensively elaborated. Our emphasis is on catalyst development. In addition, we present an outlook that summarizes the research challenges and opportunities associated with the hydrogenation of CO2 to hydrocarbon products.