文献类型：期刊文献

中文题名：退役锂离子电池湿法回收生命周期和经济评价

英文题名：Life cycle and economic assessment of recycling spent lithium-ion batteries with hydrometallurgical process

作者：周诗雨[1,2];何婷[1,2];付彤彤[1,2];郭子睿[1,2];顾帅[1,2];于建国[1,2]

机构：[1]华东理工大学国家盐湖资源综合利用工程技术研究中心,上海200237;[2]华东理工大学钾锂战略资源国际联合实验室,上海200237

年份：2023

卷号：55

期号：1

起止页码：26

中文期刊名：无机盐工业

外文期刊名：Inorganic Chemicals Industry

收录：CSTPCD;;北大核心:【北大核心2020】；CSCD:【CSCD_E2023_2024】；

基金：上海市自然科学基金(22ZR141580020);上海市青年科技英才扬帆计划项目(21YF1409000)。

语种：中文

中文关键词：退役锂离子电池;湿法回收;生命周期评价;经济性评价

外文关键词：spent lithium-ion batteries;hydrometallurgical recycling;life cycle assessment;economic assessment

摘要：锂离子电池(LIBs)具有能量密度高、输出功率大等优点被广泛应用,随之产生了大量退役LIBs。近年来,退役LIBs回收再利用逐渐受到了人们的关注,但目前回收体系尚不完善,存在发展动力和科学技术等方面的问题。从生命周期评价(LCA)和经济性评价两方面对典型的盐酸、硫酸-双氧水和电化学浸出3种回收方法进行分析讨论。使用SimaPro 9软件对回收过程进行生命周期评价,得到全球变暖潜能值、非生物资源耗竭潜能值和资源消耗量等,结果表明酸用量和能量消耗为主要的环境影响因素;并对回收再利用过程(包括预处理、浸出、再制备)进行经济性分析,得到相应的收益情况。结果表明,目前回收成本较高,整体呈现亏损状态。基于此,提出了相应的优化建议。
Lithium-ion batteries(LIBs) have been widely used because of high energy density and high output power,resulting in a large number of spent LIBs.In recent years,the recycling and utilization of spent LIBs has attracted the attention of researchers.However,the current recovery system is not perfect,due to problems in development momentum,science and technology.The three typical recovery processes,i.e.,HCl,H_(2)SO_(4)-H_(2)O_(2) and electrochemical leaching,with life cycle assessment(LCA) and economic evaluation were compared.SimaPro 9 software was used to conduct LCA on the recovery process,and obtain global warming potential value,non biological resource depletion potential value,resource consumption,etc.The results showed that acid dosage and energy consumption were the main factors determining environmental burden.Economic analysis of three recovery processes including pretreatment,leaching,and regeneration was carried to obtain the corresponding profits.The analysis found that the cost of the current recycling process was high,resulting in the deficit of the whole recycling process.Therefore,corresponding optimization suggestions were put forward.