文献类型：期刊文献

英文题名：Recent advances in photo-enhanced dry reforming of methane: A review

作者：He, Chengxuan[1];Wu, Shiqun[1];Wang, Lingzhi[1];Zhang, Jinlong[1,2]

机构：[1]East China Univ Sci & Technol, Shanghai Engn Res Ctr Multimedia Environm Catalys, Frontiers Sci Ctr Materiobiol & Dynam Chem, Key Lab Adv Mat,Sch Chem & Mol Engn, 130 Meilong Rd, Shanghai 200237, Peoples R China;[2]Yancheng Inst Technol, Sch Chem & Chem Engn, Yancheng 224051, Peoples R China

年份：2022

卷号：51

外文期刊名：JOURNAL OF PHOTOCHEMISTRY AND PHOTOBIOLOGY C-PHOTOCHEMISTRY REVIEWS

收录：;EI(收录号：20215011313402);WOS:【SCI-EXPANDED(收录号:WOS:000742849100004)】；

基金：This study was supported by National Natural Science Foundation of China (22006038, 21972040), the Program of Introducing Talents of Discipline to Universities (B20031), Innovation Program of Shanghai Municipal Education Commission (2021-01-07-00-02-E00106), the Science and Technology Commission of Shanghai Municipality (20DZ2250400) and Fundamental Research Funds for the Central Universities.

语种：英文

外文关键词：Dry reforming of methane; Carbon dioxide; Methane; Photocatalysis

摘要：Converting methane and carbon dioxide into hydrogen and carbon monoxide is significant and attractive because it can mitigate the greenhouse effect and produce useful chemical intermediate. However, these two greenhouse gases are challenging to convert due to their high bond energy and chemically inert. Although thermocatalytic dry reforming of methane (DRM) achieves high efficiency, it requires high energy and often causes deactivation due to carbon deposition. Recently, a lot of research results show that photo-enhanced DRM is a promising and green route for this reaction under relatively mild conditions. This review first introduces the importance and challenge of CH4 and CO2 conversion. Then, we summarize the related reports of photo-enhanced dry reforming of methane in detail, including material preparation, experimental conditions and results, and mechanism study. In particular, the related studies have been classified according to types of input energy and the types of catalyst. Finally, we provide insightful perspectives and prospects for the future development of this field.