文献类型：期刊文献

英文题名：CO2 capture and in-situ conversion: recent progresses and perspectives

作者：Shao, Bin[1];Zhang, Yun[1];Sun, Zheyi[1];Li, Jianping[2,3];Gao, Zihao[1];Xie, Zhicheng[1];Hu, Jun[1,2];Liu, Honglai[1]

机构：[1]East China Univ Sci & Technol, Sch Chem & Mol Engn, 130 Meilong Rd, Shanghai 200237, Peoples R China;[2]East China Univ Sci & Technol, ECUST Sch Carbon Neutral Future Technol, 130 Meilong Rd, Shanghai 200237, Peoples R China;[3]East China Univ Sci & Technol, State Environm Protect Key Lab Environm Risk Asses, 130 Meilong Rd, Shanghai 200237, Peoples R China

年份：2022

卷号：3

期号：3

起止页码：189

外文期刊名：GREEN CHEMICAL ENGINEERING

收录：EI(收录号：20224313011040);WOS:【ESCI(收录号:WOS:001072924700001)】；

基金：Acknowledgements The authors are grateful to the fi nancial support from Shanghai Sci-ence and Technology Committee (No. 19160712100) and National Natural Science Foundation of China (No. 21878076) .

语种：英文

外文关键词：CO 2 capture; In-situ conversion; Dual-function materials; Process design; Industrial applications

摘要：Global warming caused by excess carbon dioxide (CO2) emission has been a focus of the world. The development of neutral carbon technologies becomes a strategic choice for the sustainable human society. Integrating CO2 capture and conversion (iCCC) technology can simultaneously convert the captured CO2 from flue gas into valueadded chemicals, which saves great energies and expenses incurred in CO2 compression and transportation processes of conventional carbon capture, utilization, and storage (CCUS) technology. The present review critically discusses the dual-function materials (DFMs) and the iCCC technology at intermediate temperature for methane production and high temperature for syngas production. The design of reactor and optimization of operation conditions are emphasized from the perspective of industrial applications. The dual-fixed-bed reactors mode by switching the flue gas and reactant gases, and the dual-fluidized-bed reactors mode by the circulation of DFMs particles are comparatively reviewed. We hope this review can stimulate further studies including designing and fabricating feasible DFMs, exploring realistic catalytic process for CO2 conversion to high value-added chemicals, developing workable reactor modes and optimizing operation conditions, and establishing industrial demonstration for real applications of iCCC technology in the future.