文献类型：期刊文献

中文题名：东海沉积物中多溴联苯醚的分布特征研究

英文题名：The distribution of polybrominated piphenyl rther in the sediment of East China Sea

作者：周鹏[1];林匡飞[2];于慧娟[1];赵建华[2];蔡友琼[1];刘莉莉[2]

机构：[1]中国水产科学研究院东海水产研究所农业部水产品质量安全风险评估实验室,上海200090;[2]华东理工大学国家环境保护化工过程环境风险评价与控制重点实验室,上海200237

年份：2016

卷号：36

期号：1

起止页码：149

中文期刊名：中国环境科学

外文期刊名：China Environmental Science

收录：CSTPCD;;EI(收录号：20161002059056);Scopus;北大核心:【北大核心2014】；CSCD:【CSCD2015_2016】；

基金：环保公益性行业科研专项(201309047;201309030);国家自然科学基金(41001316;41371467;40901148);中央高校基本科研业务费(NO.WB1214059)

语种：中文

中文关键词：多溴联苯醚;东海;沉积物;分布;TOC

外文关键词：polybrominated diphenyl ethers; East China Sea; sediment; distribution; total organic carbon

摘要：采集分析了中国东海28个表层沉积物和7个柱状沉积物.结果表明,东海表层沉积物中除BDE-209外∑PBDEs的浓度范围为0.20~2.09ng/g dw,BDE-209的浓度范围为0.57~2.87ng/g dw,在总PBDEs中所占浓度百分比为57.9%~76.7%;接下来分别是BDE-99和BDE-47,所占比例分别为11.7%~21.5%和7.1%~17.4%.表层沉积物中PBDEs分布呈现出（离海岸线）由近及远浓度越来越低的趋势,由北到南浓度上升的趋势.东海柱状沉积物中PBDEs浓度随着深度加深呈现出先上升后下降的趋势,很好的反映出了PBDEs在中国大陆的使用历史和现状.表层沉积物TOC含量在0.54%~0.88%之间,柱状沉积物TOC的含量在0.62%~0.88%之间,而且不管是表层沉积物（R2=0.723,P〈0.01）还是柱状沉积物（R2=0.595,P〈0.01）,PBDEs浓度和TOC含量之间有较强的线性关系,表明沉积物中TOC含量是影响PBDEs分布的一个重要因素.
In this study, 28 surface sediment and 7core sediment samples were collected from the East China Sea（ECS） to determine the distribution properties of polybrominated diphenyl ethers（PBDEs）. The concentrations of total PBDEs（excepted BDE-209） in surface sediment samples were in the range of 0.20~2.09ng/g dw. Among the detected congeners, BDE-209 was the predominant congener with the corresponding concentration ranging from 0.57~2.87ng/g dw（57.9%~76.7% of total PBDEs）, followed by BDE-99 and BDE-47. Moreover, the concentrations of PBDEs decreased with the increase of distance between sampling sites and coastline and increased from the north to south. The distribution trends of PBDEs in core sediment samples from the ECS matched well with the application history and status of PBDEs products in China. The ratios of total organic carbon（TOC） in the surface and core sediment samples were ranged from 0.54%~0.88% and 0.62%~0.88% respectively. And the correlations between TOC and PBDEs in both surface（R2=0.723, P 0.01） and core（R2=0.595, P0.01） sediment samples indicated that TOC might be one of the impact factors for the characteristics of PBDEs distribution in sediment.