文献类型：期刊文献

英文题名：Recent advances in three-dimensional graphene based materials for catalysis applications

作者：Qiu, Bocheng;Xing, Mingyang[1];Zhang, Jinlong[1]

机构：[1]East China Univ Sci & Technol, Key Lab Adv Mat, 130 Meilong Rd, Shanghai 200237, Peoples R China; East China Univ Sci & Technol, Inst Fine Chem, Sch Chem & Mol Engn, 130 Meilong Rd, Shanghai 200237, Peoples R China

年份：2018

卷号：47

期号：6

起止页码：2165

外文期刊名：CHEMICAL SOCIETY REVIEWS

收录：;WOS:【SCI-EXPANDED(收录号:WOS:000429201500010)】；

基金：This work was supported by the National Natural Science Foundation of China (5171101651, 21677048, 21773062, and 21577036), State Key Research Development Program of China (2016YFA0204200), the "Chenguang Program" from Shanghai Education Development Foundation (14CG30), the Science and Technology Commission of Shanghai Municipality (16JC1401400, 17520711500), Shanghai Pujiang Program (17PJD011), and the Fundamental Research Funds for the Central Universities (22A201514021).

语种：英文

摘要：Over the past few decades, two-dimensional graphene based materials (2DGMs) have piqued the interest of scientists worldwide, and the exploration of their potential applications in catalysis, sensors, electronic devices and energy storage due to their extraordinary physical and chemical properties has rapidly progressed. As for these 2DGMs, there is a complementary need to assemble 2D building blocks hierarchically into more complicated and hierarchical three-dimensional graphene-based materials (3DGMs). Such a capability is vitally crucial in order to design sophisticated and multi-functional catalysts with tailorable properties. This comprehensive review describes some important recent advances with respect to 3DGMs, including their preparation methods, characterization and applications in catalysis, e.g., photocatalysis, electrocatalysis, organic catalysis, and CO oxidation. The importance of the relationship between the structure and catalytic performance, a topic which has become a central focus of research in order to develop high-performance catalytic systems, is discussed. Likely future developments and their associated challenges are proposed and discussed.