文献类型：期刊文献

英文题名：Crystalline graphitic carbon nitride in photocatalysis

作者：Li, Zhou[1];Ma, Liang[2];Yu, Mengxue[2];Chang, Shixin[2];Huang, Zibin[1];Cheng, Zhenmin[1];Li, Yuhan[3];Carabineiro, Sonia A. C.[4];Lv, Kangle[2]

机构：[1]East China Univ Sci & Technol, Sch Chem Engn, Shanghai 200237, Peoples R China;[2]South Cent Minzu Univ, Coll Resources & Environm, Wuhan 430074, Peoples R China;[3]Chongqing Technol & Business Univ, Engn Res Ctr Waste Oil Recovery Technol & Equipmen, Chongqing Key Lab Catalysis & New Environm Mat, Minist Educ, Chongqing 400067, Peoples R China;[4]Univ NOVA Lisboa, NOVA Sch Sci & Technol, Dept Chem, LAQV REQUIMTE, P-2829516 Caparica, Portugal

年份：2024

卷号：51

外文期刊名：SURFACES AND INTERFACES

收录：;WOS:【SCI-EXPANDED(收录号:WOS:001251454100001)】；

基金：This work was financially supported by National Natural Science Foundation of China (51672312 & 52370109) ; Hubei Provincial Natural Science Foundation and Huangshi of China (2022CFD001) ; The Fundamental Research Funds for the Central Universities of South-Central Minzu University (CZP22001 & CZZ21012) and FCT/MCTES (DOIs: 10.54499/CEECINST/00102/2018/CP1567/CT0026, 10.54499/LA/P/0008/2020, 10.54499/UIDB/50006/2020 and 10.54499/UIDP/5 0006/2020) .

语种：英文

外文关键词：Crystalline carbon nitride; Photocatalysis; Redox reaction; Modification

摘要：Crystalline graphitic carbon nitride (CCN) surpasses pristine graphitic carbon nitride (CN) in photocatalytic efficacy due to its well-organized structures that can facilitate the separation and migration of charge carriers. However, the performance improvement of CCN is hindered by limited surface adsorption and/or reaction sites. This review paper elucidates the crucial role of highly photocatalytic active CCN in addressing challenges related to energy resource depletion and environmental pollution. Initially, the synthesis procedures of CCN, such as molten-salt, solvothermal, template and self-assembly methods are concisely outlined. Subsequently, strategies for CCN modification are highlighted, including morphological control, defect engineering, composite construction and single-atom modification. Finally, the future development of CCN is outlined, addressing existing challenges and opportunities.