文献类型：期刊文献

英文题名：Direct measurement of new particle formation based on tethered airship around the top of the planetary boundary layer in eastern China

作者：Qi, Ximeng[1,2];Ding, Aijun[1,2];Nie, Wei[1,2];Chi, Xuguang[1,2];Huang, Xin[1,2];Xu, Zheng[1,2];Wang, Tianyi[1,2];Wang, Zilin[1,2];Wang, Jiaping[1,2];Sun, Peng[1,2];Zhang, Qiang[3];Huo, Juntao[4];Wang, Dongfang[4];Bian, Qinggen[4];Zhou, Lei[5];Zhang, Qing[6];Ning, Zhi[6];Fei, Dongnian[7];Xiu, Guangli[5];Fu, Qingyan[4]

机构：[1]Nanjing Univ, Sch Atmospher Sci, Joint Int Res Lab Atmospher & Earth Syst Sci, Nanjing 210023, Jiangsu, Peoples R China;[2]Jiangsu Prov Collaborat Innovat Ctr Climate Chang, Nanjing 210023, Jiangsu, Peoples R China;[3]Tsinghua Univ, Minist Educ, Key Lab Earth Syst Modeling, Dept Earth Syst Sci, Beijing 100084, Peoples R China;[4]Shanghai Environm Monitoring Ctr, 55 Sanjiang Rd, Shanghai 200235, Peoples R China;[5]East China Univ Sci & Technol, Sch Resources & Environm Engn, State Environm Protect Key Lab Environm Risk Asse, Shanghai 200237, Peoples R China;[6]Hong Kong Univ Sci & Technol, Div Environm & Sustainabiliry, Clear Water Bay, Hong Kong, Peoples R China;[7]China Elect Technol Grp Corp, Inst 38, Hefei 230088, Anhui, Peoples R China

年份：2019

卷号：209

起止页码：92

外文期刊名：ATMOSPHERIC ENVIRONMENT

收录：;EI(收录号：20191606810154);WOS:【SCI-EXPANDED(收录号:WOS:000470945900009)】；

基金：This work was supported by the Ministry of Science and Technology of the Peoples Republic of China (2016YFC0200500), the National Natural Science Foundation of China (41805101, 41725020) and Natural Science Foundation of Jiangsu Province (BK20180351).

语种：英文

外文关键词：New particle formation; Tethered airship; The top of the planetary boundary layer; Eastern China

摘要：New particle formation (NPF) is one main source of atmospheric aerosols and plays an important role in global climate by contributing up to two thirds of the atmospheric cloud condensation nuclei. Numerous studies on characteristics and mechanisms of near-surface NPF have been conducted in last decades. However, the characteristics of NPF around the top of the planetary boundary layer (PBL) remains unclear due to the limitations of vertical measurements. In this study, a tethered airship onboard with advanced particle instruments was deployed for directly measurement of the NPF exactly above and under the top of the PBL in the Yangtze River Delta (YRD) of eastern China in December 2017. Coupled with the real time ground Lidar observation, we successfully conducted measurement of aerosol size distribution, chemical components of aerosol and gas pollutants with 100 m above/under the top of the PBL. Despite not being observed within the PBL during the flight and at three ground sites in YRD, NPF event with the growth rate of 3.8 nm/h was detected above the PBL. High oxidizing capacity, enough condensable vapors and low condensation sink above the PBL favor the onset of NPF. Model simulation and the aerosol chemical composition result indicate the important role of gaseous sulfuric acid in NPF and its subsequent growth in the upper atmosphere. Our study highlights the potential mechanism of NPF above the PBL and the need of direct vertical measurements to better understand NPF in the atmosphere and its climate effect.