详细信息

Graphene-polymer reinforcement of perovskite lattices for durable solar cells  ( SCI-EXPANDED收录)  

文献类型:期刊文献

英文题名:Graphene-polymer reinforcement of perovskite lattices for durable solar cells

作者:Li, Qing[1];Zheng, Yichu[2];Wang, Haonan[1];Liu, Xinyi[1];Lin, Miaoyu[1];Sui, Xinyuan[1];Leng, Xuesong[1];Liu, Da[1];Wei, Zhanpeng[1];Song, Mengyao[1];Li, Dongdong[1];Yang, Hua Gui[1];Yang, Shuang[1];Hou, Yu[1]

机构:[1]East China Univ Sci & Technol, Shanghai Engn Res Ctr Hierarch Nanomat, Sch Mat Sci & Engn, Key Lab Ultrafine Mat,Minist Educ, Shanghai, Peoples R China;[2]Shanghai Univ, Sch Mechatron Engn & Automat, Shanghai, Peoples R China

年份:2025

卷号:387

期号:6738

起止页码:1069

外文期刊名:SCIENCE

收录:;WOS:【SCI-EXPANDED(收录号:WOS:001492007200030)】;

基金:This work was funded by the National Ten Thousand Talent Program for Young Top-notch Talent; National Natural Science Foundation of China (22379044, 52203330, 12304109); Science and Technology Commission of Shanghai Municipality (21DZ1207101, 23520710700); Key Program of the National Natural Science Foundation of China (22239001); International (Regional) Cooperation and Exchange Projects of the National Natural Science Foundation of China (51920105003); Shanghai Pilot Program for Basic Research (22TQ1400100-5); Dawn Program of Shanghai Education Commission (22SG28); Shanghai Municipal Natural Science Foundation (22ZR1418000); Shanghai Sailing Program (22YF1410000, 22YF1413100); Postdoctoral Research Foundation of China (2021M701190); Fundamental Research Funds for the Central Universities (JKD01241607, JKVD1241041); Shanghai Engineering Research Center of Hierarchical Nanomaterials (18DZ2252400); and Shanghai Frontiers Science Center of Optogenetic Techniques for Cell Metabolism (Shanghai Municipal Education Commission).

语种:英文

摘要:The lattice deformation and structural evolution of perovskite films in response to electric fields, temperature, and light limit the operational endurance of solar cells. We mechanically reinforced perovskite thin films by integrating a polymer-coupled monolithic single-layer graphene interface that led to a twofold enhancement in modulus and hardness. The synergistic effect of graphene and poly(methyl methacrylate) restricted photoinduced lattice expansion and decreased the deformation ratio from 0.31 to 0.08%, which minimized the structural damage caused by dynamic lattice evolution. Solar cell devices maintained >97% of their initial power conversion efficiency after maximum power point tracking for >3670 hours under full-spectrum air mass 1.5 global (AM 1.5 G) sunlight at 90 degrees C.

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