详细信息
Novel Ag-AgBr decorated composite membrane for dye rejection and photodegradation under visible light
文献类型:期刊文献
中文题名:Novel Ag-AgBr decorated composite membrane for dye rejection and photodegradation under visible light
作者:Yixing Wang[1];Liheng Dai[1];Kai Qu[1];Lu Qin[1];Linzhou Zhuang[1];Hu Yang[1];Zhi Xu[1]
机构:[1]State Key Laboratory of Chemical Engineering,School of Chemical Engineering,East China University of Science and Technology,Shanghai 200237,China
年份:2021
卷号:15
期号:4
起止页码:892
中文期刊名:Frontiers of Chemical Science and Engineering
外文期刊名:化学科学与工程前沿(英文版)
收录:CSTPCD;;Scopus;CSCD:【CSCD2021_2022】;PubMed;
基金:We gratefully acknowledge the financial support from the National Natural Science Foundation of China(Grant No.21908054).
语种:英文
中文关键词:Ag-AgBr;dye rejection;photodegradation;visible light
摘要:Photocatalytic membranes have received increasing attention due to their excellent separation and photodegradation of organic contaminants in wastewater.Herein,we bound Ag-AgBr nanoparticles onto a synthesized polyacrylonitrile-ethanolamine(PAN-ETA)membrane with the aid of a chitosan(CS)-TiO_(2) layer via vacuum filtration and in-situ partial reduction.The introduction of the CS-TiO_(2) layer improved surface hydrophilicity and provided attachment sites for the Ag-AgBr nanoparticles.The PAN-ETA/CS-Ti0_(2)/Ag-AgBr photocatalytic membranes showed a relatively high water permeation flux(?47 L·m^(-2)·h^(-1)·bar^(-1))and dyes rejection(methyl orange:88.22%;congo red:95%;methyl blue:97.41%;rose bengal:99.98%).Additionally,the composite membranes exhibited potential long-term stability for dye/salt separation(dye rejection:-97%;salt rejection:-6.5%).Moreover,the methylene blue and rhodamine B solutions(20 mL,10 mg·L^(-1))were degraded approximately 90.75% and 96.81% in batch mode via the synthesized photocatalytic membranes under visible light irradiation for 30 min.This study provides a feasible method for the combination of polymeric membranes and inorganic catalytic materials.
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